國立虎尾科技大學 |

Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor

Record Type:	Language materials, printed : Monograph/item
Title/Author:	Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor/ by Craig S. Slater.
Author:	Slater, Craig S.
Description:	XIII, 186 p.online resource. :
Contained By:	Springer Nature eBook
Subject:	Spectroscopy. -
Online resource:	https://doi.org/10.1007/978-3-319-24517-1
ISBN:	9783319245171

Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor
Slater, Craig S.

Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor[electronic resource] /by Craig S. Slater. - 1st ed. 2016. - XIII, 186 p.online resource. - Springer Theses, Recognizing Outstanding Ph.D. Research,2190-5053. - Springer Theses, Recognizing Outstanding Ph.D. Research,.

Introduction and Motivation -- Experimental Techniques and Methods of Data Analysis -- Three-Dimensional Velocity-Map Imaging -- Pulsed-Field Electron-Ion Imaging -- Principles of Coulomb Explosion Imaging -- Investigations of Coulomb Explosion Dynamics -- Time-resolved Studies of Induced Torsional Motion.

The work presented in this thesis involves a number of sophisticated experiments highlighting novel applications of the Pixel Imaging Mass Spectrometry (PImMS) camera in the field of photoinduced molecular dynamics. This approach represents the union of a new enabling technology (a multiple memory register, CMOS-based pixel detector) with several modern chemical physics approaches and represents a significant leap forward in capabilities. Applications demonstrated include three-dimensional imaging of photofragment Newton spheres, simultaneous electron-ion detection using a single sensor, and ion-ion velocity correlation measurements that open the door to novel covariance imaging experiments. When combined with Coulomb explosion imaging, such an approach is demonstrated to allow the measurement of molecular structure and motion on a femtosecond timescale. This is illustrated through the controlled photoexcitation of torsional motion in biphenyl molecules and the subsequent real-time measurement of the torsional angle.

ISBN: 9783319245171

Standard No.: 10.1007/978-3-319-24517-1doiSubjects--Topical Terms:

1102161
Spectroscopy.

LC Class. No.: QD95-96

Dewey Class. No.: 543.2-543.8

Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor
LDR:02786nam a22004095i 4500 001 977298
003 DE-He213
005 20200706102338.0
007 cr nn 008mamaa
008 201211s2016 gw | s |||| 0|eng d
020 $a 9783319245171 $9 978-3-319-24517-1
024 7 $a 10.1007/978-3-319-24517-1 $2 doi
035 $a 978-3-319-24517-1
050 4 $a QD95-96
072 7 $a PNFS $2 bicssc
072 7 $a SCI078000 $2 bisacsh
072 7 $a PNFS $2 thema
082 0 4 $a 543.2-543.8 $2 23
100 1 $a Slater, Craig S. $4 aut $4 http://id.loc.gov/vocabulary/relators/aut $3 1102210
245 1 0 $a Studies of Photoinduced Molecular Dynamics Using a Fast Imaging Sensor $h [electronic resource] / $c by Craig S. Slater.
250 $a 1st ed. 2016.
264 1 $a Cham : $b Springer International Publishing : $b Imprint: Springer, $c 2016.
300 $a XIII, 186 p. $b online resource.
336 $a text $b txt $2 rdacontent
337 $a computer $b c $2 rdamedia
338 $a online resource $b cr $2 rdacarrier
347 $a text file $b PDF $2 rda
490 1 $a Springer Theses, Recognizing Outstanding Ph.D. Research, $x 2190-5053
505 0 $a Introduction and Motivation -- Experimental Techniques and Methods of Data Analysis -- Three-Dimensional Velocity-Map Imaging -- Pulsed-Field Electron-Ion Imaging -- Principles of Coulomb Explosion Imaging -- Investigations of Coulomb Explosion Dynamics -- Time-resolved Studies of Induced Torsional Motion.
520 $a The work presented in this thesis involves a number of sophisticated experiments highlighting novel applications of the Pixel Imaging Mass Spectrometry (PImMS) camera in the field of photoinduced molecular dynamics. This approach represents the union of a new enabling technology (a multiple memory register, CMOS-based pixel detector) with several modern chemical physics approaches and represents a significant leap forward in capabilities. Applications demonstrated include three-dimensional imaging of photofragment Newton spheres, simultaneous electron-ion detection using a single sensor, and ion-ion velocity correlation measurements that open the door to novel covariance imaging experiments. When combined with Coulomb explosion imaging, such an approach is demonstrated to allow the measurement of molecular structure and motion on a femtosecond timescale. This is illustrated through the controlled photoexcitation of torsional motion in biphenyl molecules and the subsequent real-time measurement of the torsional angle.
650 0 $a Spectroscopy. $3 1102161
650 0 $a Physical chemistry. $3 1148725
650 0 $a Atomic structure . $3 1253596
650 0 $a Molecular structure . $3 1253597
650 1 4 $a Spectroscopy/Spectrometry. $3 782573
650 2 4 $a Physical Chemistry. $3 668972
650 2 4 $a Atomic/Molecular Structure and Spectra. $3 783942
710 2 $a SpringerLink (Online service) $3 593884
773 0 $t Springer Nature eBook
776 0 8 $i Printed edition: $z 9783319245157
776 0 8 $i Printed edition: $z 9783319245164
776 0 8 $i Printed edition: $z 9783319373911
830 0 $a Springer Theses, Recognizing Outstanding Ph.D. Research, $x 2190-5053 $3 1253569
856 4 0 $u https://doi.org/10.1007/978-3-319-24517-1
912 $a ZDB-2-CMS
912 $a ZDB-2-SXC
950 $a Chemistry and Materials Science (SpringerNature-11644)
950 $a Chemistry and Material Science (R0) (SpringerNature-43709)