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Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases

Record Type:	Language materials, printed : Monograph/item
Title/Author:	Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases/ by Cédric Schmidt.
Author:	Schmidt, Cédric.
Description:	XVI, 119 p. 40 illus., 35 illus. in color.online resource. :
Contained By:	Springer Nature eBook
Subject:	Chemistry/Food Science, general. -
Online resource:	https://doi.org/10.1007/978-3-030-67838-8
ISBN:	9783030678388

Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases
Schmidt, Cédric.

Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases[electronic resource] /by Cédric Schmidt. - 1st ed. 2021. - XVI, 119 p. 40 illus., 35 illus. in color.online resource. - Springer Theses, Recognizing Outstanding Ph.D. Research,2190-5061. - Springer Theses, Recognizing Outstanding Ph.D. Research,.

Introduction -- Theoretical Background -- Method and Setup Description -- Time-resolved XAS of Gas Dissociations -- Pulse Peak Power Optimiza@on With Filamentation.

This work studies the relaxation dynamics of molecules in both the gas and liquid phases after strong field ionization, using transient absorption in the soft X-rays. In particular, the thesis presents the first realization of time-resolved X-ray absorption spectroscopy in the spectral water window with a laser-based HHG source. These remarkable experiments were not only performed for isolated molecules, but also in liquids, for which the spectral coverage of the K-edges of C, N, and O are of primary importance for investigating biological molecules. The technique relies on the generation of high-order harmonics to further probe the electronic structure of molecules. Using the atomic selectivity of high energies and the temporal coherence of laser technology, we demonstrate the observation of the first stages of chemical transformation of matter in the gas and liquid phases. .

ISBN: 9783030678388

Standard No.: 10.1007/978-3-030-67838-8doiSubjects--Topical Terms:

593890
Chemistry/Food Science, general.

LC Class. No.: QH505

Dewey Class. No.: 571.4

Time-Resolved Soft X-Ray Absorption Spectroscopy of Molecules in the Gas and Liquid Phases
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