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Progress Toward the Total Synthesis ...

Lopez, Alberto Michael.

Progress Toward the Total Synthesis of Daphniphyllum alkaloids.

紀錄類型:	書目-語言資料,手稿 : Monograph/item
正題名/作者:	Progress Toward the Total Synthesis of Daphniphyllum alkaloids./
作者:	Lopez, Alberto Michael.
面頁冊數:	1 online resource (342 pages)
附註:	Source: Dissertation Abstracts International, Volume: 79-09(E), Section: B.
Contained By:	Dissertation Abstracts International79-09B(E).
標題:	Organic chemistry. -
電子資源:	click for full text (PQDT)
ISBN:	9780355826890

Progress Toward the Total Synthesis of Daphniphyllum alkaloids.
Lopez, Alberto Michael.

Progress Toward the Total Synthesis of Daphniphyllum alkaloids. - 1 online resource (342 pages)

Source: Dissertation Abstracts International, Volume: 79-09(E), Section: B.

Thesis (Ph.D.)--Wayne State University, 2018.

Includes bibliographical references

The Daphniphyllum alkaloids are polycyclic natural products isolated from evergreen trees and shrubs native to areas of Southeast Asia. Their structural complexity and biological activity has motived the synthetic community to devise unique strategies to access these molecules. An elegant biomimetic synthesis of methyl homodaphniphyllate by Heathcock and co-workers in 1992 was the first reported total synthesis of a Daphniphyllum alkaloid. In the years since that report, approximately 300 Daphniphyllum alkaloids have been isolated and reported. This recent flood of discovery has been met with an analogous upsurge of interest. Since 2011, 10 total syntheses and several partial syntheses of Daphniphyllum alkaloids have been reported.

Electronic reproduction.
Ann Arbor, Mich. :
ProQuest,
2018

Mode of access: World Wide Web

ISBN: 9780355826890Subjects--Topical Terms:

1148722
Organic chemistry.
Index Terms--Genre/Form:

554714
Electronic books.

Progress Toward the Total Synthesis of Daphniphyllum alkaloids.
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100 1 $a Lopez, Alberto Michael. $3 1192642
245 1 0 $a Progress Toward the Total Synthesis of Daphniphyllum alkaloids.
264 0 $c 2018
300 $a 1 online resource (342 pages)
336 $a text $b txt $2 rdacontent
337 $a computer $b c $2 rdamedia
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500 $a Source: Dissertation Abstracts International, Volume: 79-09(E), Section: B.
500 $a Adviser: Jennifer L. Stockdill.
502 $a Thesis (Ph.D.)--Wayne State University, 2018.
504 $a Includes bibliographical references
520 $a The Daphniphyllum alkaloids are polycyclic natural products isolated from evergreen trees and shrubs native to areas of Southeast Asia. Their structural complexity and biological activity has motived the synthetic community to devise unique strategies to access these molecules. An elegant biomimetic synthesis of methyl homodaphniphyllate by Heathcock and co-workers in 1992 was the first reported total synthesis of a Daphniphyllum alkaloid. In the years since that report, approximately 300 Daphniphyllum alkaloids have been isolated and reported. This recent flood of discovery has been met with an analogous upsurge of interest. Since 2011, 10 total syntheses and several partial syntheses of Daphniphyllum alkaloids have been reported.
520 $a In our retrosynthetic analysis of calyciphylline A and daphnicyclidin-type alkaloids, we imagined that a N-centered radical tandem cyclization would rapidly build their tricyclic. Indeed, this key cyclization was achieved and we were compelled to pursue the total synthesis of the target molecules.
533 $a Electronic reproduction. $b Ann Arbor, Mich. : $c ProQuest, $d 2018
538 $a Mode of access: World Wide Web
650 4 $a Organic chemistry. $3 1148722
655 7 $a Electronic books. $2 local $3 554714
690 $a 0490
710 2 $a ProQuest Information and Learning Co. $3 1178819
710 2 $a Wayne State University. $b Chemistry. $3 1192035
773 0 $t Dissertation Abstracts International $g 79-09B(E).
856 4 0 $u http://pqdd.sinica.edu.tw/twdaoapp/servlet/advanced?query=10686855 $z click for full text (PQDT)

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